Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst

Wei Fang; Chengfeng Du; Min Kuang; Mengxin Chen; Wenjing Huang; Hao Ren; Jianwei Xu; Armin Feldhoff; Qingyu Yan

doi:10.1039/d0cc01759k

Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst

Wei Fang, Chengfeng Du, Min Kuang, Mengxin Chen, Wenjing Huang, Hao Ren, Jianwei Xu^*, Armin Feldhoff, Qingyu Yan

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

66 Citations (Scopus)

Abstract

An electrochemical nitrogen oxidation approach has been realized experimentally by a Pd-decorated MXene (Ti₃C₂T_x, T = F and O) electrocatalyst under ambient conditions. The Pd-MXene catalyst can achieve a desirable nitrate yield rate of 2.80 µg h^-1mg_cat^-1(equivalent to 45.16 µmol h^-1g_cat^-1HNO₃) as well as a high nitrate faradaic efficiency of 11.34% in a favorable neutral pH environment.

Original language	English
Pages (from-to)	5779-5782
Number of pages	4
Journal	Chemical Communications
Volume	56
Issue number	43
DOIs	https://doi.org/10.1039/d0cc01759k
Publication status	Published - May 28 2020
Externally published	Yes

Bibliographical note

Publisher Copyright:
© The Royal Society of Chemistry 2020.

ASJC Scopus Subject Areas

Electronic, Optical and Magnetic Materials
Catalysis
Ceramics and Composites
General Chemistry
Surfaces, Coatings and Films
Metals and Alloys
Materials Chemistry

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abstract = "An electrochemical nitrogen oxidation approach has been realized experimentally by a Pd-decorated MXene (Ti3C2Tx, T = F and O) electrocatalyst under ambient conditions. The Pd-MXene catalyst can achieve a desirable nitrate yield rate of 2.80 µg h-1mgcat-1(equivalent to 45.16 µmol h-1gcat-1HNO3) as well as a high nitrate faradaic efficiency of 11.34\% in a favorable neutral pH environment.",

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AU - Fang, Wei

AU - Du, Chengfeng

AU - Kuang, Min

AU - Chen, Mengxin

AU - Huang, Wenjing

AU - Ren, Hao

AU - Xu, Jianwei

AU - Feldhoff, Armin

AU - Yan, Qingyu

PY - 2020/5/28

Y1 - 2020/5/28

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AB - An electrochemical nitrogen oxidation approach has been realized experimentally by a Pd-decorated MXene (Ti3C2Tx, T = F and O) electrocatalyst under ambient conditions. The Pd-MXene catalyst can achieve a desirable nitrate yield rate of 2.80 µg h-1mgcat-1(equivalent to 45.16 µmol h-1gcat-1HNO3) as well as a high nitrate faradaic efficiency of 11.34% in a favorable neutral pH environment.

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JO - Chemical Communications

JF - Chemical Communications

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Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst

Abstract

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ASJC Scopus Subject Areas

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