Femtosecond induced transparency and absorption in the extreme ultraviolet by coherent coupling of the He 2s2p (1Po) and 2p2 (1Se) double excitation states with 800 nm light

Zhi Heng Loh, Chris H. Greene, Stephen R. Leone*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

84 Citations (Scopus)

Abstract

Femtosecond high-order harmonic transient absorption spectroscopy is used to observe electromagnetically induced transparency-like behavior as well as induced absorption in the extreme ultraviolet by laser dressing of the He 2s2p (1Po) and 2p2 (1Se) double excitation states with an intense 800 nm field. Probing in the vicinity of the 1s2 → 2s2p transition at 60.15 eV reveals the formation of an Autler-Townes doublet due to coherent coupling of the double excitation states. Qualitative agreement with the experimental spectra is obtained only when optical field ionization of both double excitation states into the N = 2 continuum is included in the theoretical model. Because the Fano q-parameter of the unperturbed probe transition is finite, the laser-dressed He atom exhibits both enhanced transparency and absorption at negative and positive probe energy detunings, respectively.

Original languageEnglish
Pages (from-to)7-13
Number of pages7
JournalChemical Physics
Volume350
Issue number1-3
DOIs
Publication statusPublished - Jun 23 2008
Externally publishedYes

ASJC Scopus Subject Areas

  • General Physics and Astronomy
  • Physical and Theoretical Chemistry

Keywords

  • Autler-Townes
  • Femtosecond
  • Helium double excitation
  • High-order harmonic
  • Transient absorption

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