Flexible Piezoelectric Nanocomposite Generators Based on Formamidinium Lead Halide Perovskite Nanoparticles

Ran Ding; He Liu; Xiaoli Zhang; Juanxiu Xiao; Rahul Kishor; Huaxi Sun; Bowen Zhu; Geng Chen; Fei Gao; Xiaohua Feng; Jingsheng Chen; Xiaodong Chen; Xiaowei Sun; Yuanjin Zheng

doi:10.1002/adfm.201602634

Flexible Piezoelectric Nanocomposite Generators Based on Formamidinium Lead Halide Perovskite Nanoparticles

Ran Ding, He Liu, Xiaoli Zhang^*, Juanxiu Xiao, Rahul Kishor, Huaxi Sun, Bowen Zhu, Geng Chen, Fei Gao, Xiaohua Feng, Jingsheng Chen, Xiaodong Chen, Xiaowei Sun, Yuanjin Zheng

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

188 Citations (Scopus)

Abstract

Organic–inorganic lead halide perovskite materials have recently attracted much attention in the field of optoelectronic devices. Here, a hybrid piezoelectric nanogenerator based on a composite of piezoelectric formamidinium lead halide perovskite (FAPbBr₃) nanoparticles and polydimethylsiloxane polymer is fabricated. Piezoresponse force spectroscopy measurements reveal that the FAPbBr₃ nanoparticles contain well-developed ferroelectric properties with high piezoelectric charge coefficient (d₃₃) of 25 pmV⁻¹. The flexible device exhibits high performance with a maximum recordable piezoelectric output voltage of 8.5 V and current density of 3.8 μA cm⁻² under periodically vertical compression and release operations. The alternating energy generated from nanogenerators can be used to charge a capacitor and light up a red light-emitting diode through a bridge rectifier. This result innovatively expands the feasibility of organic–inorganic lead halide perovskite materials for application in a wide variety of high-performance energy harvesting devices.

Original language	English
Pages (from-to)	7708-7716
Number of pages	9
Journal	Advanced Functional Materials
Volume	26
Issue number	42
DOIs	https://doi.org/10.1002/adfm.201602634
Publication status	Published - Nov 8 2016
Externally published	Yes

Bibliographical note

Publisher Copyright:
© 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim

ASJC Scopus Subject Areas

Electronic, Optical and Magnetic Materials
General Chemistry
Biomaterials
General Materials Science
Condensed Matter Physics
Electrochemistry

Keywords

FAPbBr nanoparticles
organic–inorganic lead halide perovskites
piezoelectric composites
piezoelectric nanogenerators

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10.1002/adfm.201602634

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title = "Flexible Piezoelectric Nanocomposite Generators Based on Formamidinium Lead Halide Perovskite Nanoparticles",

abstract = "Organic–inorganic lead halide perovskite materials have recently attracted much attention in the field of optoelectronic devices. Here, a hybrid piezoelectric nanogenerator based on a composite of piezoelectric formamidinium lead halide perovskite (FAPbBr3) nanoparticles and polydimethylsiloxane polymer is fabricated. Piezoresponse force spectroscopy measurements reveal that the FAPbBr3 nanoparticles contain well-developed ferroelectric properties with high piezoelectric charge coefficient (d33) of 25 pmV−1. The flexible device exhibits high performance with a maximum recordable piezoelectric output voltage of 8.5 V and current density of 3.8 μA cm−2 under periodically vertical compression and release operations. The alternating energy generated from nanogenerators can be used to charge a capacitor and light up a red light-emitting diode through a bridge rectifier. This result innovatively expands the feasibility of organic–inorganic lead halide perovskite materials for application in a wide variety of high-performance energy harvesting devices.",

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AU - Ding, Ran

AU - Liu, He

AU - Zhang, Xiaoli

AU - Xiao, Juanxiu

AU - Kishor, Rahul

AU - Sun, Huaxi

AU - Zhu, Bowen

AU - Chen, Geng

AU - Gao, Fei

AU - Feng, Xiaohua

AU - Chen, Jingsheng

AU - Chen, Xiaodong

AU - Sun, Xiaowei

AU - Zheng, Yuanjin

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AB - Organic–inorganic lead halide perovskite materials have recently attracted much attention in the field of optoelectronic devices. Here, a hybrid piezoelectric nanogenerator based on a composite of piezoelectric formamidinium lead halide perovskite (FAPbBr3) nanoparticles and polydimethylsiloxane polymer is fabricated. Piezoresponse force spectroscopy measurements reveal that the FAPbBr3 nanoparticles contain well-developed ferroelectric properties with high piezoelectric charge coefficient (d33) of 25 pmV−1. The flexible device exhibits high performance with a maximum recordable piezoelectric output voltage of 8.5 V and current density of 3.8 μA cm−2 under periodically vertical compression and release operations. The alternating energy generated from nanogenerators can be used to charge a capacitor and light up a red light-emitting diode through a bridge rectifier. This result innovatively expands the feasibility of organic–inorganic lead halide perovskite materials for application in a wide variety of high-performance energy harvesting devices.

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Flexible Piezoelectric Nanocomposite Generators Based on Formamidinium Lead Halide Perovskite Nanoparticles

Abstract

Bibliographical note

ASJC Scopus Subject Areas

Keywords

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