Ionic covalent organic framework based electrolyte for fast-response ultra-low voltage electrochemical actuators

Fei Yu, Jing Hao Ciou, Shaohua Chen, Wei Church Poh, Jian Chen, Juntong Chen, Kongcharoen Haruethai, Jian Lv, Dace Gao, Pooi See Lee*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

80 Citations (Scopus)

Abstract

Electrically activated soft actuators with large deformability are important for soft robotics but enhancing durability and efficiency of electrochemical actuators is challenging. Herein, we demonstrate that the actuation performance of an ionic two-dimensional covalent-organic framework based electrochemical actuator is improved through the ordered pore structure of opening up efficient ion transport routes. Specifically, the actuator shows a large peak to peak displacement (9.3 mm, ±0.5 V, 1 Hz), a fast-response time to reach equilibrium-bending (~1 s), a correspondingly high bending strain difference (0.38%), a broad response frequency (0.1–20 Hz) and excellent durability (>99%) after 23,000 cycles. The present study ascertains the functionality of soft electrolyte as bionic artificial actuators while providing ideas for expanding the limits in applications for robots.

Original languageEnglish
Article number390
JournalNature Communications
Volume13
Issue number1
DOIs
Publication statusPublished - Dec 2022
Externally publishedYes

Bibliographical note

Publisher Copyright:
© 2022, The Author(s).

ASJC Scopus Subject Areas

  • General Chemistry
  • General Biochemistry,Genetics and Molecular Biology
  • General Physics and Astronomy

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