Polarization-Dependent Purcell Enhancement on a Two-Dimensional h-BN/WS2 Light Emitter with a Dielectric Plasmonic Nanocavity

Bowen Du, Yu Li, Meiling Jiang, Hongbo Zhang, Lishu Wu, Wen Wen, Zheng Liu*, Zheyu Fang*, Ting Yu*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

8 Citations (Scopus)

Abstract

Integrating two-dimensional (2D) transition-metal dichalcogenides (TMDCs) into dielectric plasmonic nanostructures enables the miniaturization of on-chip nanophotonic devices. Here we report on a high-quality light emitter based on the newly designed 2D h-BN/WS2 heterostructure integrated with an array of TiO2 nanostripes. Different from a traditional strongly coupled system such as the TMDCs/metallic plasmonic nanostructure, we first employ dielectric nanocavities and achieve a Purcell enhancement on the nanoscale at room temperature. Furthermore, we demonstrate that the light emission strength can be effectively controlled by tuning the polarization configuration. Such a polarization dependence meanwhile could be proof of the resonant energy transfer theory of dipole-dipole coupling between TMDCs and a dielectric nanostructure. This work gains experimental and simulated insights into modified spontaneous emission with dielectric nanoplasmonic platforms, presenting a promising route toward practical applications of 2D semiconducting photonic emitters on a silica-based chip.

Original languageEnglish
Pages (from-to)1649-1655
Number of pages7
JournalNano Letters
Volume22
Issue number4
DOIs
Publication statusPublished - Feb 23 2022
Externally publishedYes

Bibliographical note

Publisher Copyright:
© 2022 American Chemical Society

ASJC Scopus Subject Areas

  • Bioengineering
  • General Chemistry
  • General Materials Science
  • Condensed Matter Physics
  • Mechanical Engineering

Keywords

  • dielectric plasmonic nanocavity
  • energy transfer
  • exciton−plasmon coupling
  • h-BN/WS heterostructure
  • spontaneous emission

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