Abstract
Integrating two-dimensional (2D) transition-metal dichalcogenides (TMDCs) into dielectric plasmonic nanostructures enables the miniaturization of on-chip nanophotonic devices. Here we report on a high-quality light emitter based on the newly designed 2D h-BN/WS2 heterostructure integrated with an array of TiO2 nanostripes. Different from a traditional strongly coupled system such as the TMDCs/metallic plasmonic nanostructure, we first employ dielectric nanocavities and achieve a Purcell enhancement on the nanoscale at room temperature. Furthermore, we demonstrate that the light emission strength can be effectively controlled by tuning the polarization configuration. Such a polarization dependence meanwhile could be proof of the resonant energy transfer theory of dipole-dipole coupling between TMDCs and a dielectric nanostructure. This work gains experimental and simulated insights into modified spontaneous emission with dielectric nanoplasmonic platforms, presenting a promising route toward practical applications of 2D semiconducting photonic emitters on a silica-based chip.
Original language | English |
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Pages (from-to) | 1649-1655 |
Number of pages | 7 |
Journal | Nano Letters |
Volume | 22 |
Issue number | 4 |
DOIs | |
Publication status | Published - Feb 23 2022 |
Externally published | Yes |
Bibliographical note
Publisher Copyright:© 2022 American Chemical Society
ASJC Scopus Subject Areas
- Bioengineering
- General Chemistry
- General Materials Science
- Condensed Matter Physics
- Mechanical Engineering
Keywords
- dielectric plasmonic nanocavity
- energy transfer
- exciton−plasmon coupling
- h-BN/WS heterostructure
- spontaneous emission